Optimization of denoising approaches in the context of ultra-fast LIBS imaging

Guerrini, Ruggero; Alvarez-Llamas, C.; Sancey, L.; Motto-Ros, V.; Duponchel, Ludovic

Type de document :

Article dans une revue scientifique: Article original

DOI :

10.1016/j.sab.2025.107167

URL permanente :

http://hdl.handle.net/20.500.12210/126868

Titre :

Optimization of denoising approaches in the context of ultra-fast LIBS imaging

Auteur(s) :

Guerrini, Ruggero [Auteur]
Laboratoire Avancé de Spectroscopie pour les Intéractions la Réactivité et l'Environnement - UMR 8516 [LASIRE]
Alvarez-Llamas, C. [Auteur]
Institut Lumière Matière [Villeurbanne] [ILM]
Sancey, L. [Auteur]
Institute for Advanced Biosciences / Institut pour l'Avancée des Biosciences (Grenoble) [IAB]
Motto-Ros, V. [Auteur]
Institut Lumière Matière [Villeurbanne] [ILM]
Duponchel, Ludovic [Auteur]

Laboratoire Avancé de Spectroscopie pour les Intéractions la Réactivité et l'Environnement (LASIRE) - UMR 8516

Titre de la revue :

Spectroc. Acta Pt. B-Atom. Spectr.

Nom court de la revue :

Spectroc. Acta Pt. B-Atom. Spectr.

Numéro :

227

Pagination :

Date de publication :

2025-03-29

ISSN :

0584-8547

Mot(s)-clé(s) en anglais :

LIBS imaging
Denosing methods
Elemental analysis
PCA
kHz LIBS

Discipline(s) HAL :

Chimie/Chimie théorique et/ou physique

Résumé en anglais : [en]

Laser-Induced Breakdown Spectroscopy (LIBS) has emerged as a powerful analytical tool capable of providing multi-elemental information from a single laser pulse with minimal sample preparation. This technique generates a ...
Lire la suite >Laser-Induced Breakdown Spectroscopy (LIBS) has emerged as a powerful analytical tool capable of providing multi-elemental information from a single laser pulse with minimal sample preparation. This technique generates a laser-induced, transient plasma on the sample surface, whose spectral emission is analyzed to determine its elemental composition. μLIBS-Imaging, a variant offering spatially resolved elemental analysis, holds promise for applications in diverse fields such as industry, geology, forensics, and biomedicine. Our drive to go ever faster and analyze increasingly larger areas of interest in samples now compels us to use kHz lasers for this elemental imaging. Despite its potential, implementing such lasers in μLIBS-imaging would face diverse challenges mainly related to weak plasma emission and signal-to-noise ratio (SNR) degradation, particularly when applied to delicate biological samples. This paper investigates methods to enhance SNR in fast μLIBS imaging, particularly for biomedical applications. We focus on denoising techniques suitable for high-frequency laser applications, comparing methods like Savitzky-Golay smoothing, Fast Fourier Transform, wavelet-based filtering, Whittaker Filtering, and Principal Component Analysis (PCA). Our strategy optimizes denoising parameters for specific elemental emission peaks, enhancing SNR for individual elements of interest. The results demonstrate significant improvements in data quality, paving the way for more accurate and efficient elemental imaging in complex biomedical specimens.Lire moins >

Langue :

Anglais

Audience :

Internationale

Vulgarisation :

Non

Établissement(s) :

Université de Lille
CNRS

Collections :

Laboratoire Avancé de Spectroscopie pour les Intéractions la Réactivité et l'Environnement (LASIRE) - UMR 8516

Date de dépôt :

2025-04-05T21:02:00Z
2025-04-16T08:06:11Z

Numéro de version	Lien	Date de modification
2	20.500.12210/126868*	2025-04-16T08:03:48Z
1	20.500.12210/126868.1	2025-04-05T21:02:00Z

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